반응 #81111

ord-f0ac4d596dbe41c58ce781b429bc5435

반응 조건

상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    온도The reaction mixture was warmed at 50° C. for 5 hours
  2. 2
    온도re-cooled to -20° C.
  3. 3
    온도The reaction mixture was heated an additional 2.5 hours at 50° C.
  4. 4
    농축concentrated under reduced pressure
  5. 5
    기타to afford an amorphous solid
  6. 6
    기타The solid was triturated with ether

실험 절차

To anhydrous methanol (15 mL) at -20° C. under nitrogen was added thionyl chloride (4 mL) dropwise. The solution was allowed to warm to room temperature and then tert-Leucine (4.00 g) was added. The reaction mixture was warmed at 50° C. for 5 hours, re-cooled to -20° C. and then additional thionyl chloride (3 mL) was added dropwise. The reaction mixture was heated an additional 2.5 hours at 50° C. and then concentrated under reduced pressure and chased twice with methanol (15 mL) to afford an amorphous solid. The solid was triturated with ether to afford the title compound in 92% yield. The 300 MHz 1H NMR spectrum was found to be consistent with the proposed structure. MS (DCI/NH3) m/e 146 (M+H)+.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US05616714uspto-grants-1997_04