반응 #77736

ord-dc86013d85064869934468b248415d6a

반응 조건

상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    온도The mixture is heated
  2. 2
    온도at reflux temperature for 1.5 h
  3. 3
    추출extracted with ethyl acetate
  4. 4
    농축concentrated in vacuo
  5. 5
    기타to afford an oily residue
  6. 6
    온도heated
  7. 7
    온도at reflux temperature overnight
  8. 8
    온도cooled to 0° C. for several hours
  9. 9
    여과filtered
  10. 10
    기타The filtercake is dried

실험 절차

A solution of N-(4-acetyl-3-hydroxyphenyl)acetamide (4.00 g., 21 mmol) and diethyl oxalate (7.3 mL, 54 mmol) in absolute ethanol is added dropwise to a solution of sodium ethoxide (0.1 mol) in absolute ethanol. The mixture is heated at reflux temperature for 1.5 h, cooled to ambient temperature, poured into water, acidified to pH 3 with 6N HCl and extracted with ethyl acetate. The extracts are combined and concentrated in vacuo to afford an oily residue. The residue is dissolved in ethanol, treated with concentrated HCl heated at reflux temperature overnight, cooled to 0° C. for several hours and filtered. The filtercake is dried to afford the title compound as an orange solid, 2.95 g (61% yield), mp 195°-198° C., identified by NMR and mass spectral analyses.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US06706757B2uspto-grants-2004_03