반응 #443155

ord-e7d4f75550c041269b4deeaf859b8d30

반응 조건

상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    workup.STIRRINGAfter stirring for 20 minutes
  2. 2
    추출The chloroform layer was extracted
  3. 3
    농축concentrated
  4. 4
    workup.ADDITIONTo the concentrate were added 20 ml of toluene
  5. 5
    온도by heating
  6. 6
    온도under reflux for 1 hour
  7. 7
    workup.ADDITIONUpon addition of 100 ml of ethyl acetate
  8. 8
    세척the reaction product was washed with saturated brine
  9. 9
    건조dried over anhydrous sodium sulfate
  10. 10
    기타The solvent was evaporated
  11. 11
    workup.DISSOLUTIONthe residue was dissolved into a mixed solvent of 20 ml of ethanol, 20 ml of dioxane, and 0.2 ml of acetic acid
  12. 12
    workup.ADDITIONThe mixture was catalytically hydrogenated with the addition of 200 mg of platinum oxide
  13. 13
    기타The catalyst was removed
  14. 14
    농축the filtrate was concentrated
  15. 15
    workup.ADDITIONether was added to the concentrate

실험 절차

The compound obtained in (5) above (1 gm) was dissolved into 20 ml of ethanol. To the solution was added 166 mg of sodium borohydride while stirring at room temperature. After stirring for 20 minutes, chloroform and 10% citric acid were added to the reaction mixture. The chloroform layer was extracted and concentrated. To the concentrate were added 20 ml of toluene and a small amount of p-TsOH, followed by heating under reflux for 1 hour. Upon addition of 100 ml of ethyl acetate, the reaction product was washed with saturated brine and dried over anhydrous sodium sulfate. The solvent was evaporated and the residue was dissolved into a mixed solvent of 20 ml of ethanol, 20 ml of dioxane, and 0.2 ml of acetic acid. The mixture was catalytically hydrogenated with the addition of 200 mg of platinum oxide. The catalyst was removed, the filtrate was concentrated, and ether was added to the concentrate. 0.8 gm of the title compound was obtained by collecting the precipitate by filtration.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US05834476uspto-grants-1998_11