반응 #332116

ord-6240f5aad3754305a4564a1319224a31

반응 방정식

CC(C)C(=O)Cl
isobutyryl chloride
CC(C)NC(C)C.[Li]
lithiumdiisopropylamine
CCCCCCc1ccc(CC(=O)OCC)cc1
ethyl 2-(4-hexylphenyl)acetate
CCCCCCc1ccc(C(C(=O)OCC)C(=O)C(C)C)cc1
desired product
수율 70.5%
CCCCCCc1ccc(C(C(=O)OCC)C(=O)C(C)C)cc1
ethyl 2-(4-hexylphenyl)-4-methyl-3-oxopentanoate
수율 70.5%

반응 조건

온도
-60°CELSIUS
상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    온도the solution was warmed to 0° C.
  2. 2
    온도The reactuion solution was cooled to −60° C. again
  3. 3
    기타The reaction was quenched with saturated aqueous sodium hydrogen carbonate (150 ml)
  4. 4
    추출the reaction solution was extracted with ethyl acetate
  5. 5
    건조The organic layer was dried over anhydrous magnesium sulfate
  6. 6
    여과filtered
  7. 7
    농축the filtrate was concentrated under reduced pressure
  8. 8
    기타The resulting residue was purified by silica gel column chromatography

실험 절차

6.0 g (24 mmol) of ethyl 2-(4-hexylphenyl)acetate was dissolved in 130 mL of dry tetrahydrofuran under a nitrogen atmosphere and cooled to −60° C. After addition of 31.8 mL (36.2 mmol) of 1.14 M solution of lithiumdiisopropylamine in hexane/tetrahydrofuran, the solution was warmed to 0° C. and stirred for 1 hours. The reactuion solution was cooled to −60° C. again and stirred with 3.6 g (34 mmol) of isobutyryl chloride at −60° C. to room temperature for 15 hours. The reaction was quenched with saturated aqueous sodium hydrogen carbonate (150 ml), and the reaction solution was extracted with ethyl acetate. The organic layer was dried over anhydrous magnesium sulfate and filtered, and the filtrate was concentrated under reduced pressure. The resulting residue was purified by silica gel column chromatography using ethyl acetate:hexane (0:100 to 1:9) as the eluent to give 5.39 g of the desired product as a pale yellw oil.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US08658686B2uspto-grants-2014_02