반응 #2879

ord-6f47bc261884491694bca9fab87d052d

반응 조건

온도
80°CELSIUS
상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    온도the mixture was cooled to about 55° C.
  2. 2
    온도The resulting mixture was heated to 80° C
  3. 3
    기타was consumed
  4. 4
    기타Upon complete reaction
  5. 5
    온도to cool to room temperature
  6. 6
    농축the organic layer concentrated in vacuo at 40° C.
  7. 7
    기타The resulting oil was used in the next step without further purification

실험 절차

A mixture of ethyl 4-hydroxybenzoate (8.31 g), 1-(2-chloroethyl)piperidine monohydrochloride (10.13 g), potassium carbonate (16.59 g), and methyl ethyl ketone (60 mL) was heated to 80° C. After one hour, the mixture was cooled to about 55° C. and treated with additional 1-(2-chloroethyl)piperidine mono-hydrochloride (0.92 g). The resulting mixture was heated to 80° C. The reaction was monitored by thin layer chromatography (TLC), using silica-gel plates and ethyl acetate/acetonitrile/triethylamine (10:6:1, v/v). Additional portions of 1-(2-chloroethyl)piperidine hydrochloride were added until the starting 4-hydroxybenzoate ester was consumed. Upon complete reaction, the reaction mixture was treated with water (60 mL) and allowed to cool to room temperature. The aqueous layer was discarded and the organic layer concentrated in vacuo at 40° C. and 40 mm Hg. The resulting oil was used in the next step without further purification.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US05731327uspto-grants-1998_03