반응 #170212

ord-e39f36dbb045417292916c9bd246c6b5

반응 조건

상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    기타then partitioned between ethyl acetate (30 mL) and water (30 mL)
  2. 2
    기타The aqueous layer was separated
  3. 3
    추출finally extracted with ethyl acetate (2×50 mL)
  4. 4
    세척The combined organic phases were washed with a saturated solution of sodium chloride (3×50 mL)
  5. 5
    건조dried over sodium sulfate
  6. 6
    농축concentrated to dryness
  7. 7
    기타The residue was purified by chromatography on silica gel

실험 절차

3-(Thiophen-2-ylmethoxy)-azetidine hydrochloride (61 mg, 0.30 mmol), EDCI (71.5 mg, 0.37 mmol), HOBt (52 mg, 0.37 mmol) and diisopropylethylamine (110 μL, 0.62 mmol) were successively added to a solution of (E)-3-(3-((dimethylamino)methyl)-1H-pyrrolo[2,3-b]pyridin-5-yl)acrylic acid hydrochloride (70 mg, 0.25 mmol) in dimethylformamide (10 mL) at room temperature. The reaction mixture was stirred overnight then partitioned between ethyl acetate (30 mL) and water (30 mL). The aqueous layer was separated, basified with an aqueous solution of sodium hydroxyde (2N) until pH 12 and finally extracted with ethyl acetate (2×50 mL). The combined organic phases were washed with a saturated solution of sodium chloride (3×50 mL), dried over sodium sulfate and concentrated to dryness. The residue was purified by chromatography on silica gel using dichloromethane/methanol/ammoniac (1:0:0.1 to 9:1:0.1) as eluent. The title product was obtained as a yellow solid (10 mg, 10%).

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US08846711B2uspto-grants-2014_09