반응 #156201

ord-5ebe8529af324a4c958c08808cf03096

반응 조건

온도
60°CELSIUS
상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    온도The reaction mixture was cooled to room temperature
  2. 2
    workup.STIRRINGstirred at 60° C. for 24 hours
  3. 3
    추출the extraction with ethyl acetate
  4. 4
    세척The organic layer was washed with a saturated sodium chloride aqueous solution
  5. 5
    건조dried over anhydrous sodium sulfate
  6. 6
    농축concentrated under reduced pressure
  7. 7
    기타The residue was purified by silica gel column chromatography (n-hexane:ethyl acetate=1:1→0:1)
  8. 8
    기타condensed under reduced pressure
  9. 9
    workup.STIRRINGthe liquid was stirred at room temperature
  10. 10
    기타The precipitated insoluble product was separated
  11. 11
    세척washed with ether
  12. 12
    기타dried

실험 절차

Sodium iodide (113 mg) was added to a DMF solution (5 ml) of N-(3-chloropropyl)-N-(2-methylbenzyl)-N-(2-pyridin-3-ylethyl)amine (151 mg), and stirred at 60° C. for 1 hours. The reaction mixture was cooled to room temperature. Potassium carbonate (104 mg) and 6-hydroxyquinoline (87 mg) were then added to the reaction mixture and stirred at 60° C. for 24 hours. The reaction mixture was added to ice water, and the extraction with ethyl acetate was performed. The organic layer was washed with a saturated sodium chloride aqueous solution, dried over anhydrous sodium sulfate, and concentrated under reduced pressure. The residue was purified by silica gel column chromatography (n-hexane:ethyl acetate=1:1→0:1). The purified product was condensed under reduced pressure. A 4N-hydrogen chloride in ethyl acetate solution (0.014 ml) was added to a ethyl acetate solution (1 ml) of the residue, and the liquid was stirred at room temperature. The precipitated insoluble product was separated, washed with ether, and dried to give the title compound (7.6 mg) as a brown powder.

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US08822453B2uspto-grants-2014_09