반응 #1277449

ord-10d61e4f0b35443ea6b8be07a10ea958

반응 조건

온도
2.5°CELSIUS
상세 조건
See reaction.notes.procedure_details.

후처리

  1. 1
    기타After removal of the solvents
  2. 2
    기타the residue was partitioned between ethyl acetate and saturated sodium carbonate aqueous solution
  3. 3
    세척The organic layer was washed with water, brine
  4. 4
    건조dried over sodium sulfate
  5. 5
    여과After filtration
  6. 6
    농축the filtrate was concentrated

실험 절차

9-Chloro-4,5-dihydro-6-oxa-1-thia-10-aza-benzo[e]azulene (4.33 g, 18.2 mmol) was dissolved in methylene chloride (40 mL, 600 mmol)/acetic acid (40 mL, 700 mmol). The solution was cooled down to 0-5° C. and added a solution of N-Bromosuccinimide (3.57 g, 20.0 mmol) in 10 mL of DCM slowly. The reaction mixture was stirred for 18 hours. After removal of the solvents, the residue was partitioned between ethyl acetate and saturated sodium carbonate aqueous solution. The organic layer was washed with water, brine and dried over sodium sulfate. After filtration, the filtrate was concentrated to give 2-Bromo-9-chloro-4,5-dihydro-6-oxa-1-thia-10-aza-benzo[e]azulene. 1HNMR (DMSO, 400 MHz): δ 7.48 (d, J=8.4 Hz, 1H, ArH), 7.28 (d, J=8.4 Hz, 1H, ArH), 7.18 (s, 1H, ═CH), 4.32 (t, J=4.4 Hz, 2H, CH2), 3.17 (t, J=4.4 Hz, 2H, CH2).

출처

DOI: 10.6084/m9.figshare.5104873.v1특허: US08673952B2uspto-grants-2014_03