反応 #77402

ord-e4e7aca93424416bbe838ccfee595aab

反応条件

温度
100°CELSIUS
詳細条件
See reaction.notes.procedure_details.

後処理

  1. 1
    温度The mixture was cooled to room temperature
  2. 2
    温度The mixture was heated at 100° C. for 2 hours
  3. 3
    温度cooled
  4. 4
    その他quenched with 300 mL of saturated ammonium chloride solution
  5. 5
    抽出The mixture was extracted three times with ethyl acetate
  6. 6
    洗浄the combined organic layers were washed with water and brine
  7. 7
    その他evaporated

実験手順

Dimethyl malonate (10 mL) in 25 mL of dimethylsulfoxide was added dropwise to 3.5 g of sodium hydride suspended in 25 mL of dimethylsulfoxide and the mixture heated at 100° C. for 10 minutes. The mixture was cooled to room temperature and 4.7 g of 4-fluoro-3-nitrobiphenyl in 25 mL of dimethylsulfoxide was added. The mixture was heated at 100° C. for 2 hours, cooled and quenched with 300 mL of saturated ammonium chloride solution. The mixture was extracted three times with ethyl acetate and the combined organic layers were washed with water and brine and evaporated to give crude dimethyl-3-nitrobiphenyl-4-malonate as a yellow oil.

出典

DOI: 10.6084/m9.figshare.5104873.v1特許: US06706709B2uspto-grants-2004_03