反応 #55080

ord-80bb9ca87dee465e97accc18056e570b

反応条件

詳細条件
See reaction.notes.procedure_details.

後処理

  1. 1
    温度The mixture is heated
  2. 2
    温度under reflux for 4 hours
  3. 3
    洗浄washed with water and with dilute bicarbonate solution
  4. 4
    その他dried
  5. 5
    その他The mixture is evaporated in vacuo
  6. 6
    その他After leaving the reactants in contact overnight
  7. 7
    その他the mixture is evaporated to dryness in vacuo
  8. 8
    ろ過the mixture is filtered over charcoal
  9. 9
    その他the filtrate is precipitated with 3 N HCl
  10. 10
    抽出the product is extracted with ether
  11. 11
    その他the extract is dried
  12. 12
    その他evaporated
  13. 13
    その他the product is crystallised in diisopropyl ether

実験手順

20.2 g (0.08 mol) of 3,4-dichlorobenzylthioacetic acid are esterified with 10 ml of methanol, 0.6 ml of concentrated H2SO4 and 100 ml of dichloroethane. The mixture is heated under reflux for 4 hours, washed with water and with dilute bicarbonate solution, and dried. The mixture is evaporated in vacuo. The oily residue, in methanol, is treated with a solution of hydroxylamine (0.1 mol) in the presence of 0.18 mol of sodium methylate. After leaving the reactants in contact overnight, the mixture is evaporated to dryness in vacuo, the residue is taken up in water, the mixture is filtered over charcoal and the filtrate is precipitated with 3 N HCl, the product is extracted with ether, the extract is dried and evaporated and the product is crystallised in diisopropyl ether. 15 g of the stated product are obtained (yield 71%). Melting point: 75°-76° C.

出典

DOI: 10.6084/m9.figshare.5104873.v1特許: US04151300uspto-grants-1979_04