反応 #50721

ord-30ae960048bd4360a69c341e55ed4e51

反応方程式

C=C(C)c1ccccc1C
isopropenyltoluene
[Na+].[OH-]
NaOH
C=C(C)c1ccccc1C
isopropenyltoluene
C1=Cc2ccccc2C1
indene
C1=Cc2ccccc2C1
indene
FB(F)F.[O-]c1ccccc1
boron trifluoride phenolate
C1=Cc2ccccc2C1.C=C(C)c1ccccc1C
isopropenyltoluene indene

反応条件

詳細条件
See reaction.notes.procedure_details.

後処理

  1. 1
    その他t-he polymerization reaction
  2. 2
    その他was carried out at a reaction temperature of 5° C
  3. 3
    その他the polymerization reaction at 5° C
  4. 4
    その他the polymerization reaction
  5. 5
    その他After the polymerization
  6. 6
    その他the polymerization reaction
  7. 7
    その他The obtained reaction mixture
  8. 8
    洗浄was washed 5 times with large amounts of water
  9. 9
    workup.DISTILLATIONThen, the solvent and the unreacted monomer were distilled off in an evaporator under a reduced pressure

実験手順

In all of these Examples, an autoclave equipped with stirrer vanes and having a real content of 1270 ml was continuously served with an isopropenyltoluene, an indene, a dehydrated and refined toluene and a boron trifluoride phenolate complex (phenol, 1.6 times equivalent) diluted 10-fold with the dehydrated and refined toluene at ratios as shown in Table 1, so that the total amount of the isopropenyltoluene and the indene was 1.0 l/hr, and t-he polymerization reaction was carried out at a reaction temperature of 5° C. The reaction mixture was then shifted to an autoclave of the second stage to continue the polymerization reaction at 5° C. When the total residence time in the autoclaves of the first and second stages has reached two hours, the reaction mixture was continuously discharged, and the polymerization reaction was finished when three times of the residence time has passed. After the polymerization, a 1N NaOH aqueous solution was added to the reaction mixture to stop the polymerization reaction. The obtained reaction mixture was washed 5 times with large amounts of water. Then, the solvent and the unreacted monomer were distilled off in an evaporator under a reduced pressure to obtain an isopropenyltoluene/indene copolymer. The polymerization conditions(monomer feeding ratio, amount of catalyst, resin composition, yield) were as shown in Table 1. Properties (hue, softening point, molecular weight Mw, Tg, melt viscosity) of the obtained isopropenyltoluene/-indene copolymer resin were measured in compliance with the methods described below. The results were as shown in Table 2.

出典

DOI: 10.6084/m9.figshare.5104873.v1特許: US05428109uspto-grants-1995_06