反応 #367587

ord-02593f30af49449aad3b58787b0a4074

反応方程式

O=C(O)CCCCC(=O)O
adipic acid
CC=CCC(=O)N(CC)CC
pent-3-enoic acid diethylamide
CC=CCC(=O)N(CC)CC
pent-3-enoic acid diethylamide
CCO
ethanol
CCC=CC(=O)N(CC)CC
pentenoic acid diethylamide
CCCCC(=O)N(CC)CC
n-pentanoic acid diethylamide

溶媒

反応条件

詳細条件
See reaction.notes.procedure_details.

後処理

  1. 1
    温度After cooling
  2. 2
    その他had been formed

実験手順

77.6 g of pent-3-enoic acid diethylamide, 32.2 g of ethanol, 1.58 g of pyridine and 3.42 g of Co2 (CO)8 were reacted, as described in Example 1, for 1 hour at 170° C. under a carbon monoxide pressure of 150 bar (+approx. 2% by volume of H2). After cooling, analysis indicated a conversion of pent-3-enoic acid diethylamide of 47.3 mol %. Relative to this, 61.5 mol % of C6 -dicarboxylic acid ethylester-diethylamides had been formed and these had the following composition: 64.6% (=I1) of 2-ethylsuccinic acid 1-ethylester-4-diethylamide, 29.2% of 2-methylglutaric acid 1-ethylester-5-diethylamide and 6.2% of adipic acid ethylesterdiethylamide. Furthermore, as well as isomers of pentenoic acid diethylamide, n-pentanoic acid diethylamide and C6 -dicarboxylic acid bisdiethylamides (3 isomers) were formed at selectivities of conversion of 1.7 mol % and 1.1 mol %, respectively.

出典

DOI: 10.6084/m9.figshare.5104873.v1特許: US04588833uspto-grants-1986_05