反応 #1140292

ord-545f8c81172446aeb28a245d4fbf82f5

反応条件

温度
100°CELSIUS
詳細条件
See reaction.notes.procedure_details.

後処理

  1. 1
    その他The reaction mixture was degassed with argon for 20 min
  2. 2
    抽出extracted with ethyl acetate (2×150 mL) and organic layer
  3. 3
    洗浄was washed with brine
  4. 4
    乾燥dried over anhydrous sodium sulphate
  5. 5
    濃縮concentrated under reduced pressure
  6. 6
    その他to get crude product
  7. 7
    その他The crude compound was purified by column chromatography
  8. 8
    洗浄was eluted with 40% ethyl acetate in petroleum ether
  9. 9
    その他to afford 500 mg, which
  10. 10
    その他was further purified
  11. 11
    洗浄by washing with diethyl ether and hexane

実験手順

To a solution of 4-[5-(2-amino-5-bromo-pyridin-3-yl)-[1,3,4]oxadiazol-2-yl]-piperidine-1-carboxylic acid tert-butyl ester (1.0 g, 2.35 mmol) in dioxane (20 mL) and water (20 mL) were added K2CO3 (0.95 g, 7.05 mmol), 3-methoxyphenyl boronic acid (0.39 g, 2.59 mmol) in a sealed tube. The reaction mixture was degassed with argon for 20 min, then Pd(PPh3)4 (0.13 g, 0.11 mmol) was added to the reaction mixture. The reaction mixture was stirred for 18 h at 100° C. The reaction mixture was diluted with water (100 mL) extracted with ethyl acetate (2×150 mL) and organic layer was washed with brine, dried over anhydrous sodium sulphate and concentrated under reduced pressure to get crude product. The crude compound was purified by column chromatography using 100-200 mesh silica gel and compound was eluted with 40% ethyl acetate in petroleum ether to afford 500 mg, which was further purified by washing with diethyl ether and hexane to afford the title compound as a pale yellow solid.

出典

DOI: 10.6084/m9.figshare.5104873.v1特許: US09393248B1uspto-grants-2016_07