Reacción #2028071

ord-564dcfae0a3f459a83c031a0c2306f9a

Ecuación de reacción

Cc1cccnc1
3-methylpyridine
CC(=O)O
acetic acid
O=C(O)c1cccnc1
nicotinic acid

Disolventes

Condiciones de reacción

Condiciones detalladas
See reaction.notes.procedure_details.

Tratamiento posterior

  1. 1
    Otroto react in the same manner as in Example 1

Procedimiento

The same autoclave as that used in Example 1 was charged with 25 parts by weight of 3-methylpyridine, 0.38 part by weight of cobalt acetate, 0.27 part by weight of manganese acetate, 1 part by weight of tetrapropylammonium bromide and 150 parts by weight of acetic acid having a 5 wt % water content, and the mixture was allowed to react in the same manner as in Example 1 to give 21.7 parts by weight of a crude nicotinic acid crystal. The conversion of the 3-methylpyridine was 93.7 mol %, the selectivity to the nicotinic acid was 99.0 mol %, and the yield of the nicotinic acid 92.8 mol %. The conversion and the yield in Example 2 were improved over those in Example 1 since the solvent was used in a larger amount in Example 2. The crude nicotinic acid had a bromine concentration of 608 ppm and showed a dissolved b value of 5.44.

Fuente

DOI: 10.6084/m9.figshare.5104873.v1Patente: US05700944uspto-grants-1997_12