Reaktion #9836

ord-bd8297b3cf7f4124a97a04ca91aa86e8

Reaktionsgleichung

O=O
oxygen
CC(=O)O
acetic acid
O=c1n(O)c(=O)n(O)c(=O)n1O
hexahydro-1,3,5-trihydroxy-1,3,5-triazine-2,4,6-trione
Cc1ccc(C(=O)O)cc1
p-toluic acid
O=C(O)c1ccc(C(=O)O)cc1
terephthalic acid
Cc1ccc(C(=O)O)cc1
p-toluic acid

Lösungsmittel

Reaktionsbedingungen

Temperatur
150°CELSIUS
Detaillierte Bedingungen
See reaction.notes.procedure_details.

Aufarbeitung

  1. 1
    Sonstigeplaced in a heated oil bath
  2. 2
    SonstigeAfter the completion of the reaction
  3. 3
    Temperaturto cool down the reaction mixture quickly

Vorschrift

In a 500-ml titanium autoclave equipped with a stirrer and a pressure gauge, 15.36 g of p-toluic acid, 104.0 g of acetic acid, 0.066 g of hexahydro-1,3,5-trihydroxy-1,3,5-triazine-2,4,6-trione (1,3,5-trihydroxyisocyanuric acid) (0.33% by mole relative to p-toluic acid), 0.112 g of cobalt(II) acetate.4H2O and 0.277 g of manganese(II) acetate.4H2O were placed. The autoclave was charged with 2 MPa of oxygen gas and 2 MPa of nitrogen gas and placed in a heated oil bath. The mixture was stirred at 150° C. for 1 hour. After the completion of the reaction, the autoclave was placed on cold water to cool down the reaction mixture quickly. The resulting mixture was analyzed by high performance liquid chromatography and was found to yield terephthalic acid in 63% yield at 68% conversion of p-toluic acid.

Quelle

DOI: 10.6084/m9.figshare.5104873.v1Patent: US07091342B2uspto-grants-2006_08