Reaktion #5859

ord-6c9c4dc14ecb42679eca1006ffa0ee05

Reaktionsgleichung

O=P([O-])([O-])[O-].[NH4+].[NH4+].[NH4+]
ammonium phosphate
O=[N+]([O-])[O-].O=[N+]([O-])[O-].O=[N+]([O-])[O-].[Al+3]
aluminum nitrate
[Cl-].[Cl-].[Mg+2]
magnesium chloride
[NH4+].[OH-]
ammonium hydroxide
[Cl][Ti]([Cl])([Cl])[Cl]
TiCl4
[Cl][Ti]([Cl])([Cl])[Cl]
TiCl4
O=P([O-])([O-])[O-].[Al+3].[Mg+2]
aluminum-magnesium phosphate
[Cl][Ti]([Cl])([Cl])[Cl]
TiCl4

Lösungsmittel

Reaktionsbedingungen

Detaillierte Bedingungen
See reaction.notes.procedure_details.

Vorschrift

A series of catalysts comprising TiCl4 and a particulate cogelled xerogel of aluminum-magnesium phosphate was prepared at a pH of about 6-10 by combining aqueous solutions of aluminum nitrate, magnesium chloride, monobasic ammonium phosphate and ammonium hydroxide. Generally, each catalyst was made by slurrying the gel in n-heptane, adding sufficient TiCl4 to obtain the desired weight ratio of TiCl4 to gel, i.e., a weight ratio within the range of from about 0.4:1 to about 1.4:1, refluxing the mixture for about 30 minutes and cooling to about room temperature. Supernatant liquid was decanted, the slurry was washed with n-heptane to remove unreacted TiCl4 and the solvent was removed from the catalyst by evaporation in a dry box under nitrogen or argon.

Quelle

DOI: 10.6084/m9.figshare.5104873.v1Patent: US05246900uspto-grants-1993_09