Reaktion #1702024

ord-a0e4f3e74c53462898db953c8a49c170

Reaktionsgleichung

O=C(O)c1cccc(C(=O)O)c1
isophthalic acid
Nc1ccccc1O
aminophenol
O=C(O)c1ccc2cc(O)ccc2c1
2-hydroxy-6-naphthoic acid
CC(=O)OC(C)=O
acetic anhydride
O=C1C=CC(=O)N1
maleimide
O=C(O)c1ccccc1N1C(=O)C=CC1=O
maleimidobenzoic acid
O=C(O)c1ccccc1
benzoic acid
C#C.O=C(O)c1ccccc1
acetylene benzoic acid

Reaktionsbedingungen

Temperatur
320°CELSIUS
Detaillierte Bedingungen
See reaction.notes.procedure_details.

Aufarbeitung

  1. 1
    SonstigeAlternatively, the liquid crystalline thermoset oligomer can be prepared by a bulk polymerization process in accordance with the following procedure
  2. 2
    Temperaturto reflux for a predetermined time period
  3. 3
    SonstigeAcetic acid as a by-product and unreacted acetic anhydride are removed from the reaction mixture
  4. 4
    workup.ADDITIONNext, 4-hydroxybenzoic acid is added
  5. 5
    Temperaturthe reaction temperature is maintained which
  6. 6
    Sonstigethe reaction
  7. 7
    Sonstigeto give a liquid crystal oligomer

Vorschrift

Alternatively, the liquid crystalline thermoset oligomer can be prepared by a bulk polymerization process in accordance with the following procedure. In another exemplary method, isophthalic acid, aminophenol, 2-hydroxy-6-naphthoic acid and acetic anhydride are slowly heated to 150° C. with stirring in a reactor. The mixture is brought to reflux for a predetermined time period. Acetic acid as a by-product and unreacted acetic anhydride are removed from the reaction mixture. Next, 4-hydroxybenzoic acid is added, and the temperature is further raised to 320° C. and the reaction temperature is maintained which allows the reaction to proceed, to give a liquid crystal oligomer having one or two terminal alcohol groups at one or both ends of the backbone. The liquid crystal oligomer is dissolved in a proper solvent (e.g., N,N-dimethylformamide, abbreviated “DMF”), and then a compound (e.g., maleimidobenzoic acid, nadimide benzoic acid, or acetylene benzoic acid) capable of providing thermally crosslinkable reactive groups (e.g., maleimide, nadimide or acetylene groups) is added to the solution. The mixture is allowed to react to give the liquid crystalline thermoset oligomer having one or two thermally crosslinkable reactive groups at one or both ends of the backbone thereof.

Quelle

DOI: 10.6084/m9.figshare.5104873.v1Patent: US08765012B2uspto-grants-2014_07