Reaktion #1153184

ord-5f40991ae4fb4b4da2749d0a5b2ed208

Reaktionsgleichung

CC(=O)CCCC(C)CCCC(C)CCCC(C)C
6,10,14-trimethyl pentadecan-2-one
CC(C)=CCCC(C)=CCCC(C)=CCO
farnesol
CC(C)=CCCC(C)=CCCC(C)=CCO
Farnesol
CC(C)=CCC/C(C)=C/CC/C(C)=C/C=O
farnesal
[C-]#[C-]
acetylide
CC(=O)CCCC(C)CCCC(C)CCCC(C)C
ketone
CC(=O)CCCC(C)CCCC(C)CCCC(C)C
6,10,14-trimethyl pentadecan-2-one
CC(C)[O-].CC(C)[O-].CC(C)[O-].[Al+3]
aluminum isopropoxide
CC(C)=CCC/C(C)=C/CC/C(C)=C/C=O
Farnesal
CC(C)=CCC/C(C)=C/CC/C(C)=C/C=O
farnesal
C=CC(C)(O)CCCC(C)CCCC(C)CCCC(C)C
isophytol

Lösungsmittel

Reaktionsbedingungen

Detaillierte Bedingungen
See reaction.notes.procedure_details.

Vorschrift

A particularly preferred embodiment of synthesizing vitamin E from farnesol is illustrated in FIG. 3. Farnesol 3-8 is oxidized to farnesal 3-9 under Oppenauer oxidation conditionS using aluminum isopropoxide and acetone. Farnesal 3-9 is then converted to dehydrofarnesyl acetone 3-10 by an aldol condensation reaction with acetone. Reduction of olefin moieties on dehydrofarnesyl acetone 3-10 by hydrogenation then produces 6,10,14-trimethyl pentadecan-2-one 3-11. Addition of acetylide to the ketone 3-11 then generates propargylic alcohol 3-12 which is partially reduced using Lindlar hydrogenation condition to produce isophytol 3-13. Reaction of isophytol 3-13 with 2,3,5-trimethyl hydroquinone 3-5 in the presence of an acid catalyst then produces vitamin E.

Quelle

DOI: 10.6084/m9.figshare.5104873.v1Patent: US06242227B1uspto-grants-2001_06