تفاعل #81111

ord-f0ac4d596dbe41c58ce781b429bc5435

الكواشف

لا شيء

ظروف التفاعل

الظروف التفصيلية
See reaction.notes.procedure_details.

المعالجة

  1. 1
    درجة الحرارةThe reaction mixture was warmed at 50° C. for 5 hours
  2. 2
    درجة الحرارةre-cooled to -20° C.
  3. 3
    درجة الحرارةThe reaction mixture was heated an additional 2.5 hours at 50° C.
  4. 4
    تركيزconcentrated under reduced pressure
  5. 5
    أخرىto afford an amorphous solid
  6. 6
    أخرىThe solid was triturated with ether

الإجراء التجريبي

To anhydrous methanol (15 mL) at -20° C. under nitrogen was added thionyl chloride (4 mL) dropwise. The solution was allowed to warm to room temperature and then tert-Leucine (4.00 g) was added. The reaction mixture was warmed at 50° C. for 5 hours, re-cooled to -20° C. and then additional thionyl chloride (3 mL) was added dropwise. The reaction mixture was heated an additional 2.5 hours at 50° C. and then concentrated under reduced pressure and chased twice with methanol (15 mL) to afford an amorphous solid. The solid was triturated with ether to afford the title compound in 92% yield. The 300 MHz 1H NMR spectrum was found to be consistent with the proposed structure. MS (DCI/NH3) m/e 146 (M+H)+.

المصدر

DOI: 10.6084/m9.figshare.5104873.v1براءة الاختراع: US05616714uspto-grants-1997_04