تفاعل #6086

ord-b2df1b2c03444a26b30ca461acdd85d7

المذيبات

ظروف التفاعل

الظروف التفصيلية
See reaction.notes.procedure_details.

المعالجة

  1. 1
    أخرىfitted with a mechanical stirrer, a reflux condenser
  2. 2
    أخرىprotected by a drying tube
  3. 3
    أخرىprotected by a drying tube
  4. 4
    درجة الحرارةThe flask is cooled in an ice-bath
  5. 5
    أخرىThe cooling bath is then removed
  6. 6
    درجة الحرارةthe mixture heated
  7. 7
    درجة الحرارةat reflux for 3 hours
  8. 8
    درجة الحرارةThe mixture is then cooled in an ice-salt bath
  9. 9
    workup.ADDITION5 ml of saturated ammonium chloride solution is added
  10. 10
    ترشيحfiltered
  11. 11
    غسيلthe residue washed with two 10 ml portions of ether
  12. 12
    أخرىThe ether solution is then separated
  13. 13
    تجفيفdried (MgSO4)
  14. 14
    أخرىthe ether removed in vacuo
  15. 15
    أخرىThe residue is then purified by chromatography
  16. 16
    أخرىfollowed by recrystallization

الإجراء التجريبي

Four ml of a 3M (12 mmol) solution of ethylmagnesium bromide in ether is placed in a 3-necked flask fitted with a mechanical stirrer, a reflux condenser protected by a drying tube and a pressure-equalizing dropping funnel protected by a drying tube. The flask is cooled in an ice-bath and a solution of 3.174 g (10 mmol) of 2-[2-(5,5,8,8-tetramethyl-5,6,7,8-tetrahydronaphth-2-yl)ethynyl]pyridine-5-carboxaldehyde in 10 ml of dry ether is added slowly with vigorous stirring. The cooling bath is then removed and the mixture heated at reflux for 3 hours. The mixture is then cooled in an ice-salt bath and 5 ml of saturated ammonium chloride solution is added. The mixture is stirred for a further 1 hour and then filtered and the residue washed with two 10 ml portions of ether. The ether solution is then separated, dried (MgSO4) and the ether removed in vacuo. The residue is then purified by chromatography followed by recrystallization to give the title compound.

المصدر

DOI: 10.6084/m9.figshare.5104873.v1براءة الاختراع: US05246962uspto-grants-1993_09