تفاعل #56459

ord-abd2d97cd76d49eabf871b9bb464d08c

الكواشف

لا شيء

المذيبات

ظروف التفاعل

الظروف التفصيلية
See reaction.notes.procedure_details.

المعالجة

  1. 1
    درجة الحرارةThe mixture is heated to 50°-60° C.
  2. 2
    درجة الحرارةThe mixture is heated
  3. 3
    درجة الحرارةunder reflux
  4. 4
    درجة الحرارةboiling is maintained for 15 minutes
  5. 5
    درجة الحرارةThe mixture is cooled
  6. 6
    درجة الحرارةThe mixture is again heated
  7. 7
    درجة الحرارةunder reflux for 30 minutes
  8. 8
    درجة الحرارةcooled
  9. 9
    أخرىat 60°-70° C
  10. 10
    درجة الحرارةThe whole is then heated
  11. 11
    درجة الحرارةunder reflux for 30 minutes
  12. 12
    درجة الحرارةcooled
  13. 13
    ترشيحfiltered
  14. 14
    أخرىthe precipitate obtained
  15. 15
    ترشيحis filtered off the redissolved cold in dilute sodium bicarbonate solution
  16. 16
    غسيلthis solution is washed with methylene chloride
  17. 17
    ترشيحfiltered

الإجراء التجريبي

15.2 g (0.2 mol) of thiourea in 100 ml of water are introduced into a 1 liter 3-necked flask. The mixture is heated to 50°-60° C. and 39.1 g (0.2 mol) of 2,4-dichlorobenzylchloride are introduced in a single operation. The mixture is heated under reflux and boiling is maintained for 15 minutes; the solution becomes limpid. The mixture is cooled and a solution of 32 g (0.8 mol) of NaOH in 50 ml of water is introduced dropwise at about 60° C. The mixture is again heated under reflux for 30 minutes, cooled and a solution of about 0.28 mol of sodium chloroacetate (obtained by neutralising 26.46 g of chloroacetic acid in 200 ml of water with 23.52 g of NaHCO3) is introduced, dropwise, at 60°-70° C. The whole is then heated under reflux for 30 minutes, cooled, filtered and acidified with 3 N HCl; the precipitate obtained is filtered off the redissolved cold in dilute sodium bicarbonate solution, and this solution is washed with methylene chloride, filtered and again acidified. 41.7 g (yield: 83 %) of product are thus collected. Instantaneous melting point: 72°-73° C.

المصدر

DOI: 10.6084/m9.figshare.5104873.v1براءة الاختراع: US04225617uspto-grants-1980_09