تفاعل #51592

ord-b63b76bfbdd54ee487c6ba2080b6a6a2

معادلة التفاعل

N#CCCCCC#N
adiponitrile
N
ammonia
[H][H]
hydrogen
[Al+3].[Al+3].[O-2].[O-2].[O-2]
aluminum oxide
O=[Si]=O
silicon dioxide
[Ca+2].[O-2]
calcium oxide
NCCCCCCN
hexamethylenediamine
المردود 98.1%
NC1CCCCC1N
1,2-diaminocyclohexane

ظروف التفاعل

الظروف التفصيلية
See reaction.notes.procedure_details.

الإجراء التجريبي

DE-A-2 429 293 discloses in Example 1 that the hydrogenation of adiponitrile in the presence of five times the weight of ammonia at from 93 to 98° C. (inlet temperature into the reactor) or at from 94 to 104° C. (outlet temperature) over an iron catalyst prepared from magnetite by reduction with hydrogen and doped with aluminum oxide, silicon dioxide, calcium oxide and vanadium pentoxide yields 98.22% of hexamethylenediamine comprising 1900 ppm of 1,2-diaminocyclohexane, and in Example 2 that the hydrogenation of adiponitrile in the presence of five times the weight of ammonia at from 93 to 98° C. (inlet temperature into the reactor) or at from 94 to 104° C. (outlet temperature) over an iron catalyst prepared from Labrador hematite ore (Fe2O3) by reduction with hydrogen and doped with aluminum oxide, silicon dioxide and calcium oxide yields 98.05% of hexamethylenediamine comprising 3500 ppm of 1,2-diaminocyclohexane.

المصدر

DOI: 10.6084/m9.figshare.5104873.v1براءة الاختراع: US06852669B2uspto-grants-2005_02