تفاعل #1985946

ord-94763bb1c83c48a3b83869585f59d137

معادلة التفاعل

COC(=O)CCc1cc(O)c(OC)cc1CO[Si](C)(C)C(C)(C)C
methyl 5-hydroxy-2-tert-butyldimethylsilyloxymethyl-4-methoxyhydrocinnamate
C1CCOC1
THF
c1ccc(P(c2ccccc2)c2ccccc2)cc1
triphenylphosphine
BrC(Br)(Br)Br
carbon tetrabromide
COC(=O)CCc1cc(OC(C)=O)c(OC)cc1CBr
desired product
COC(=O)CCc1cc(OC(C)=O)c(OC)cc1CBr
Methyl 5-Acetoxy-2-bromomethyl-4-methoxyhydrocinnamate

المذيبات

ظروف التفاعل

الظروف التفصيلية
See reaction.notes.procedure_details.

المعالجة

  1. 1
    ترشيحfiltered
  2. 2
    تركيزThe filtrate is concentrated in vacuo
  3. 3
    ترشيحthe residue purified by filtration through silica gel in 50% ethyl acetate in hexanes
  4. 4
    غسيلeluting with 25% ethyl acetate in hexanes

الإجراء التجريبي

To a solution of methyl 5-hydroxy-2-tert-butyldimethylsilyloxymethyl-4-methoxyhydrocinnamate (5.21 g) in carbon tetrabromide (12.35 g) in anhydrous ether (75 ml) and anhydrous THF (50 ml) is added portionwise triphenylphosphine (9.78 g) and the mixture stirred at room temperature for 60 minutes, diluted with ether, then filtered. The filtrate is concentrated in vacuo and the residue purified by filtration through silica gel in 50% ethyl acetate in hexanes followed by HPLC, eluting with 25% ethyl acetate in hexanes, to give the desired product.

المصدر

DOI: 10.6084/m9.figshare.5104873.v1براءة الاختراع: US05571506uspto-grants-1996_11